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Abstract: Metal–organic framework-derived graphitic porous nanoribbons anchored on graphene sheets are developed as an efficient electrode for electroionic artificial muscles. The soft actuator exhibits breakthrough bending displacement (17.4 mm), very fast rise time (700 ms),wide frequency response (0.1– 15 Hz),and excellent cycling stability (92% retention after 25 000 cycles) even at 0.5 V input. The actuator was used for successful demonstration of biomimicked Venus flytrap.